Onihei's an episodic show set in the Edo period of Japan mostly focusing on the head officer of arson and theft control, pretty much dealing with him taking down criminals and dealing with his family life along the way. It has a pretty interesting cast of characters and isn't too continuity heavy. The later half of the series was probably my favourite for how intense and dramatic it got.
I liked Gargoyle and Captain Nemo the most myself, though Marie's episode did legit make me cry.
Oh, very nice! I really liked season 1 of Psycho-Pass myself, but never got around to the movie or season 2, now that I have my Netflix account back though, maybe I'll see if it's on there or Crunchyroll.
I'm currently watching season 2 of Baki, and I forgot how much fun it was. In between that I'm watching an anime called Arrow Emblem Grand Prix no Taka, which...well, this video explains it better than I could:
https://www.youtube.com/watch?v=OKygs4SGCL4